The present study deals with droplet sizing based on laser-induced fluorescence (LIF) andMie scattering for varied
polarization of the utilized laser (parallel or perpendicular). The polarization-dependent LIF/Mie ratio is studied
for micrometric droplets (25–60 m) produced with a droplet generator. The investigations were carried out with
the dyeNile red dissolved in ethanol and ethanol/iso-octane mixtures. A spectral absorption and fluorescence characterization
at various dye and ethanol concentrations is carried out in a cuvette in order to identify reabsorption
effects. The LIFjj droplet images (index jj: parallel polarization) show a more homogeneous intensity distribution
in the droplets and slightly stronger morphology-dependent resonances (MDRs) in comparison to LIF? (index?:
perpendicular polarization). The spectral LIF emissions reveal a dependence of the MDR on the ethanol admixture.
The larger the ethanol content, the lower the MDR peak, which is also shifted further to the red part of the
spectrum. TheMie droplet signal images are mainly characterized by two distinct glare points, one at the entrance
of the laser light (reflection) and one at the exit (first-order refraction). TheMie? images show a more pronounced
entrance glare point, in comparison to Miejj, where the exit glare point is more pronounced. These observations
are in accordance with the theory. The calibration curve of the micro droplet signals revealed a volumetric trend of
the LIF signals and a slightly higher LIF? signal and sensitivity in comparison to LIFjj. The signal Mie? follows
roughly a quadratic trend on average, whileMiejj follows a linear trend. Consequently, the calculated LIF?=Mie?
ratio shows a linear trend, whereas the LIFjj=Miejj ratio shows a quadratic trend, which confirms theoretical calculations.
A numerical simulation of the Mie signal at various detection angles shows a good agreement with the
experimental data at large apertures.
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